Date of Graduation
8-2025
Document Type
Thesis
Degree Name
Master of Science in Physics (MS)
Degree Level
Graduate
Department
Physics
Advisor/Mentor
Churchill, Hugh
Committee Member
Nakamura, Hiro
Second Committee Member
Hu, Jin
Keywords
Direct Band Gap; Optoelectronics; Quantum Emitter; Single Photon Emission; Strain engineering; WSe2
Abstract
Strain induced defects in monolayer tungsten diselenide (WSe₂) give rise to localized exciton funnels, offering a promising approach for the development of tunable quantum emitters. The quantum devices fabricated for this thesis used a modified dimple dot geometry, in which nano indentation creates a strain profile on the monolayer WSe₂. This allows for the funneling of excitons to a confined region. These strain induced funnels enable localized emission from single excitons in WSe₂. Device fabrication was carried out through mechanical exfoliation, dry transfer, and electron beam lithography of Cr/Au gates on a SiO₂ substrate. These devices were then characterized using atomic force microscopy (AFM), photoluminescence (PL) spectroscopy, and Stark shift measurements under applied gate voltages. Optical spectroscopy at room temperature revealed localized emission features and early indications of electric gate tunability. Dimple dot devices in WSe₂ represent a promising platform for the deterministic placement and control of quantum emitters for integrated quantum photonics applications.
Citation
Kitterman, G. M. (2025). Strain Induced Quantum Emitters in Monolayer WSe₂: Fabrication and Characterization of Dimple Dot Devices. Graduate Theses and Dissertations Retrieved from https://scholarworks.uark.edu/etd/5943